The mother-of-six may have landed just a few days ago, but Angelina was already keen to take her brood out to explore the city's attractions.
She expertly took the hands of her five-year-old twins Knox and Vivienne as she walked around the Aquarium, while her older children, Zahara, eight, Shiloh, seven, Pax, 10 and 12-year-old Maddox, followed close by.
Angelina was all smiles as she and her offspring enjoyed a fun-filled day out, and picked up some matching toy souvenirs for Zahara and Vivienne.
Angelina's new tattoo sits below her inking of the word "determination" in Arabic
The globe-trotting family often relocate for Brad and Angelina's film work. In 2012, they stayed at the £10million Wentworth Estate in Surrey, near London, while Angelina filmed Maleficent and Brad worked on scenes for The Counselor as well as parts of World War Z.
It has also been reported that the Hollywood power couple will return to the UK next year while Brad films the sequel to the post-apocalyptic thriller.